Efficient Separation of Ethanol-Methanol and Ethanol-Water Mixtures Using ZIF-8 Supported on a Hierarchical Porous Mixed-Oxide Substrate.
Identifieur interne : 000996 ( Main/Exploration ); précédent : 000995; suivant : 000997Efficient Separation of Ethanol-Methanol and Ethanol-Water Mixtures Using ZIF-8 Supported on a Hierarchical Porous Mixed-Oxide Substrate.
Auteurs : Yiwen Tang [Pays-Bas] ; David Dubbeldam [Pays-Bas] ; Xingmei Guo [République populaire de Chine] ; Gadi Rothenberg [Pays-Bas] ; Stefania Tanase [Pays-Bas]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2019.
Abstract
This work reports a new approach for the synthesis of a zeolitic imidazolate framework (ZIF-8) composite. It employs the direct growth of the crystalline ZIF-8 on a mixed-metal oxide support TiO2-SiO2 (TSO), which mimics the porous structure of Populus nigra. Using the natural leaf as a template, the TSO support was prepared using a sol-gel method. The growth of the ZIF-8 layer on the TSO support was carried out by the seeds and second growth method. This method facilitates the homogeneous dispersion of ZIF-8 crystals at the surface of the TSO composite. The ZIF-8@TSO composite adsorbs methanol selectively, mainly due to the hierarchical porous structure of the mixed oxide support. As compared with the as-synthesized ZIF-8, a 50% methanol uptake is achieved in the ZIF-8@TSO composite, with only 25 wt % ZIF-8 loading. IAST simulations show that the ZIF-8@TSO composite has a preferential adsorption toward methanol when using an equimolar methanol-ethanol mixture. An opposite behavior is observed for the as-synthesized ZIF-8. The results show that combining MOFs and mixed-oxide supports with bioinspired structures opens opportunities for synthesizing new materials with unique and enhanced adsorption and separation properties.
DOI: 10.1021/acsami.9b02325
PubMed: 31117427
PubMed Central: PMC6567680
Affiliations:
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Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author><author><name sortKey="Guo, Xingmei" sort="Guo, Xingmei" uniqKey="Guo X" first="Xingmei" last="Guo">Xingmei Guo</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental and Chemical Engineering , Jiangsu University of Science and Technology , No. 2 Mengxi Road , Zhenjiang 212003 , Jiangsu , China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Environmental and Chemical Engineering , Jiangsu University of Science and Technology , No. 2 Mengxi Road , Zhenjiang 212003 , Jiangsu </wicri:regionArea><wicri:noRegion>Jiangsu </wicri:noRegion></affiliation></author><author><name sortKey="Rothenberg, Gadi" sort="Rothenberg, Gadi" uniqKey="Rothenberg G" first="Gadi" last="Rothenberg">Gadi Rothenberg</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author><author><name sortKey="Tanase, Stefania" sort="Tanase, Stefania" uniqKey="Tanase S" first="Stefania" last="Tanase">Stefania Tanase</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country 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Supported on a Hierarchical Porous Mixed-Oxide Substrate.</title><author><name sortKey="Tang, Yiwen" sort="Tang, Yiwen" uniqKey="Tang Y" first="Yiwen" last="Tang">Yiwen Tang</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author><author><name sortKey="Dubbeldam, David" sort="Dubbeldam, David" uniqKey="Dubbeldam D" first="David" last="Dubbeldam">David Dubbeldam</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author><author><name sortKey="Guo, Xingmei" sort="Guo, Xingmei" uniqKey="Guo X" first="Xingmei" last="Guo">Xingmei Guo</name><affiliation wicri:level="1"><nlm:affiliation>School of Environmental and Chemical Engineering , Jiangsu University of Science and Technology , No. 2 Mengxi Road , Zhenjiang 212003 , Jiangsu , China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Environmental and Chemical Engineering , Jiangsu University of Science and Technology , No. 2 Mengxi Road , Zhenjiang 212003 , Jiangsu </wicri:regionArea><wicri:noRegion>Jiangsu </wicri:noRegion></affiliation></author><author><name sortKey="Rothenberg, Gadi" sort="Rothenberg, Gadi" uniqKey="Rothenberg G" first="Gadi" last="Rothenberg">Gadi Rothenberg</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author><author><name sortKey="Tanase, Stefania" sort="Tanase, Stefania" uniqKey="Tanase S" first="Stefania" last="Tanase">Stefania Tanase</name><affiliation wicri:level="1"><nlm:affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</nlm:affiliation><country xml:lang="fr">Pays-Bas</country><wicri:regionArea>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam </wicri:regionArea><wicri:noRegion>1098 XH Amsterdam </wicri:noRegion></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2019" type="published">2019</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">This work reports a new approach for the synthesis of a zeolitic imidazolate framework (ZIF-8) composite. It employs the direct growth of the crystalline ZIF-8 on a mixed-metal oxide support TiO<sub>2</sub>-SiO<sub>2</sub> (TSO), which mimics the porous structure of Populus nigra. Using the natural leaf as a template, the TSO support was prepared using a sol-gel method. The growth of the ZIF-8 layer on the TSO support was carried out by the seeds and second growth method. This method facilitates the homogeneous dispersion of ZIF-8 crystals at the surface of the TSO composite. The ZIF-8@TSO composite adsorbs methanol selectively, mainly due to the hierarchical porous structure of the mixed oxide support. As compared with the as-synthesized ZIF-8, a 50% methanol uptake is achieved in the ZIF-8@TSO composite, with only 25 wt % ZIF-8 loading. IAST simulations show that the ZIF-8@TSO composite has a preferential adsorption toward methanol when using an equimolar methanol-ethanol mixture. An opposite behavior is observed for the as-synthesized ZIF-8. The results show that combining MOFs and mixed-oxide supports with bioinspired structures opens opportunities for synthesizing new materials with unique and enhanced adsorption and separation properties.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">31117427</PMID><DateRevised><Year>2020</Year><Month>02</Month><Day>25</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1944-8252</ISSN><JournalIssue CitedMedium="Internet"><Volume>11</Volume><Issue>23</Issue><PubDate><Year>2019</Year><Month>Jun</Month><Day>12</Day></PubDate></JournalIssue><Title>ACS applied materials & interfaces</Title><ISOAbbreviation>ACS Appl Mater Interfaces</ISOAbbreviation></Journal><ArticleTitle>Efficient Separation of Ethanol-Methanol and Ethanol-Water Mixtures Using ZIF-8 Supported on a Hierarchical Porous Mixed-Oxide Substrate.</ArticleTitle><Pagination><MedlinePgn>21126-21136</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/acsami.9b02325</ELocationID><Abstract><AbstractText>This work reports a new approach for the synthesis of a zeolitic imidazolate framework (ZIF-8) composite. It employs the direct growth of the crystalline ZIF-8 on a mixed-metal oxide support TiO<sub>2</sub>-SiO<sub>2</sub> (TSO), which mimics the porous structure of Populus nigra. Using the natural leaf as a template, the TSO support was prepared using a sol-gel method. The growth of the ZIF-8 layer on the TSO support was carried out by the seeds and second growth method. This method facilitates the homogeneous dispersion of ZIF-8 crystals at the surface of the TSO composite. The ZIF-8@TSO composite adsorbs methanol selectively, mainly due to the hierarchical porous structure of the mixed oxide support. As compared with the as-synthesized ZIF-8, a 50% methanol uptake is achieved in the ZIF-8@TSO composite, with only 25 wt % ZIF-8 loading. IAST simulations show that the ZIF-8@TSO composite has a preferential adsorption toward methanol when using an equimolar methanol-ethanol mixture. An opposite behavior is observed for the as-synthesized ZIF-8. The results show that combining MOFs and mixed-oxide supports with bioinspired structures opens opportunities for synthesizing new materials with unique and enhanced adsorption and separation properties.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Tang</LastName><ForeName>Yiwen</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Dubbeldam</LastName><ForeName>David</ForeName><Initials>D</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-4382-1509</Identifier><AffiliationInfo><Affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Guo</LastName><ForeName>Xingmei</ForeName><Initials>X</Initials><AffiliationInfo><Affiliation>School of Environmental and Chemical Engineering , Jiangsu University of Science and Technology , No. 2 Mengxi Road , Zhenjiang 212003 , Jiangsu , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Rothenberg</LastName><ForeName>Gadi</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tanase</LastName><ForeName>Stefania</ForeName><Initials>S</Initials><Identifier Source="ORCID">http://orcid.org/0000-0003-2830-1924</Identifier><AffiliationInfo><Affiliation>Van't Hoff Institute for Molecular Sciences , University of Amsterdam , Science Park 904 , 1098 XH Amsterdam , The Netherlands.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2019</Year><Month>06</Month><Day>03</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Appl Mater Interfaces</MedlineTA><NlmUniqueID>101504991</NlmUniqueID><ISSNLinking>1944-8244</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">ZIF-8</Keyword><Keyword MajorTopicYN="N">adsorption</Keyword><Keyword MajorTopicYN="N">artificial leaf</Keyword><Keyword MajorTopicYN="N">composite</Keyword><Keyword MajorTopicYN="N">hierarchical system</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="pubmed"><Year>2019</Year><Month>5</Month><Day>24</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate 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last="Rothenberg">Gadi Rothenberg</name><name sortKey="Tanase, Stefania" sort="Tanase, Stefania" uniqKey="Tanase S" first="Stefania" last="Tanase">Stefania Tanase</name></country><country name="République populaire de Chine"><noRegion><name sortKey="Guo, Xingmei" sort="Guo, Xingmei" uniqKey="Guo X" first="Xingmei" last="Guo">Xingmei Guo</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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